Any alloy will
harden with age at room temp, especially if it has any traces of copper, magnesium zinc or IIRC silicon - there may be more elements.
Mag wheels, race flywheels etc - the billets are left out in the weather for years before being machined.
I have a photo somewhere where I was at a top Japanese racecar workshop, and out the back they would have had 500 billets sitting in the weather aging - been there for 5 years
My understanding through limited japanese/chinglish communication that it was for stress relief and hardening.
Copper and brass thats left for a long time will
anneal very slowly at room temp, add heat and the process is sped up.
Consider brass cases, in which get harder when fired and requires heat (annealing) to bring them back to required neck tension etc - but you're adding heat when firing each time which should make them softer...... but the working of the brass make is harder - moreso than the effect of the heat softening
As you can see, the above statements contradict each other somewhat.
I dont know/remember much more technically about it - I'm sure there is heaps of info on the net about age hardening of alloys
I have spoken with someone that agreed with your findings of a box of bulk projectiles that had sat on the window ledge in the shed for years.
Over time they shot worse and performed worse on animals - as if they were harder.
How old are the projs? maybe the deer are evolving and getting softer??
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